It depends on what kind of anime style you are trying to achieve. Visual Style was created to specifically recreate the style of Japanese Visual Novels first and formost, with many presets with soft colours and coloured outlines. Visual Style can be further edited to achieve something closer to an OVA anime style (which you seem to be going for in these renders). A user example of how this looks can be seen here:
http://iroha.b.dlsite.net/archives/1565398.html
And here is my own attempt at recreating an OVA style image someone showed me (which I don’t have on me unfortunately, so I can’t show a comparison):
http://imgur.com/2vyor
However, Visual Style does lack the ability to create even width outlines, a feature that is exclusive to PWToon.